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Query: EC:6.2.1.1 (
ACS
)
78,556
document(s) hit in 31,850,051 MEDLINE articles (0.00 seconds)
The three-dimensional (3D) structural design of solar evaporators has been considered as one of the most promising approaches toward enhancing photothermal performance by improving light absorption and the available evaporation area. Herein, polypyrrole-decorated 3D array structural sunflower discs (PPy-SFD) were prepared for solar steam generation, thereby turning
SFD
biomass waste into valuable materials. The
SFD
can absorb a majority of the incident light because of numerous light reflections from each natural 3D array structural unit, and therefore behaves similar to a blackbody. Moreover, a facile pyrrole polymerization method was introduced to further improve
SFD
light absorption and enhance the photothermal performance of
SFD
. This circumvents expensive consumption fabrication processes. The black PPy-decorated
SFD
shows a light absorption of 99.3% across the entire solar spectrum coupled with mechanical stability. During photothermal evaporation, the increased evaporation area of the 3D array structural
SFD
could effectively reduce heat loss to the environment because the inherent microporous structure of the
SFD
leaves and cellulose hydrophilicity provide channels for water transport. The PPy-
SFD
-based evaporator could reach an evaporation rate of 1.74 kg m
-2
h
-1
under 1 sun. Thus, the 3D array structural PPy-
SFD
is a possible candidate for high-efficiency photothermal evaporators.
ACS
Appl Mater Interfaces 2020 Oct 14
PMID:Blackbody-Inspired Array Structural Polypyrrole-Sunflower Disc with Extremely High Light Absorption for Efficient Photothermal Evaporation. 3294 Sep 97